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F Raulin P Coll N Smith Y Benilan P Bruston M C Gazeau 《Advances in Space Research (includes Cospar's Information Bulletin, Space Research Today)》1999,24(4):453-460
Titan, the largest satellite of Saturn, with a dense atmosphere very rich in organics, and many couplings in the various parts of its "geofluid", is a reference for studying prebiotic chemistry on a planetary scale. New data have been obtained from experiments simulating this organic chemistry (gas and aerosol phases), within the right ranges of temperature and a careful avoiding of any chemical contamination. They show a very good agreement with the observational data, demonstrating for the first time the formation of all the organic species already detected in Titan atmosphere including, at last, C4N2, together with many other species not yet detected in Titan. This strongly suggests the presence of more complex organics in Titan's atmosphere and surface, including high molecular weight polyynes and cyanopolyynes. The NASA-ESA Cassini-Huygens mission has been successfully launched in October 1997. The Cassini spacecraft will reach the Saturn system in 2004 and become an orbiter around Saturn, while the Huygens probe will penetrate into Titan's atmosphere. In situ measurements, in particular from Huygens GC-MS and ACP instruments, will provide a detailed analysis of the organics present in the air, aerosols, and surface. This very ambitious mission should yield much information of crucial importance for our knowledge of the complexity of Titan's chemistry, and, more generally for the field of exobiology. 相似文献
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S I Ramirez R Navarro-Gonzalez P Coll F Raulin 《Advances in Space Research (includes Cospar's Information Bulletin, Space Research Today)》2001,27(2):261-270
A quantitative comparison of the products arising from the irradiation of a Titan's simulated atmosphere is presented. The energy sources used represent some of the main events that occur in the satellite's atmosphere. All of the compounds identified are classified in the hydrocarbon and nitrile chemical families. Almost all of the detected compounds in Titan's atmosphere are produced by one or more energy sources. The compounds with the highest energy yields include the C2 hydrocarbons, methanonitrile and ethanonitrile. The possibility of using some of the produced organics as tracer compounds during the Huygens descend to identify the leading energy form in the different atmospheric levels remains open. 相似文献
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H2O2-PE固液火箭发动机低频不稳定燃烧研究 总被引:3,自引:0,他引:3
介绍了85%H2O2-PE固液火箭发动机的低频不稳定燃烧特征;应用发动机质量守恒方程对发动机低频耦合振荡燃烧现象进行了一维模拟,分析了氧化剂喷射压降对低频不稳定燃烧的影响。利用扰动分析确立了固液火箭发动机的稳定工作限。提出了抑制低频耦合振荡燃烧的方法。 相似文献
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Cottin H Guan YY Noblet A Poch O Saiagh K Cloix M Macari F Jérome M Coll P Raulin F Stalport F Szopa C Bertrand M Chabin A Westall F Chaput D Demets R Brack A 《Astrobiology》2012,12(5):412-425
The PROCESS (PRebiotic Organic ChEmistry on the Space Station) experiment was part of the EXPOSE-E payload outside the European Columbus module of the International Space Station from February 2008 to August 2009. During this interval, organic samples were exposed to space conditions to simulate their evolution in various astrophysical environments. The samples used represent organic species related to the evolution of organic matter on the small bodies of the Solar System (carbonaceous asteroids and comets), the photolysis of methane in the atmosphere of Titan, and the search for organic matter at the surface of Mars. This paper describes the hardware developed for this experiment as well as the results for the glycine solid-phase samples and the gas-phase samples that were used with regard to the atmosphere of Titan. Lessons learned from this experiment are also presented for future low-Earth orbit astrochemistry investigations. 相似文献
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P Coll D Coscia M C Gazeau E de Vanssay J C Guillemin F Raulin 《Advances in Space Research (includes Cospar's Information Bulletin, Space Research Today)》1995,16(2):93-103
Many experiments have already been carried out to simulate organic chemistry on Titan, the largest satellite of Saturn. They can provide fruitful information on the nature of minor organic constituents likely to be present in Titan's atmosphere, both in gas and aerosol phases. Indeed, all the organic compounds but one already detected in Titan's atmosphere have been identified in simulation experiments. The exception, C4N2, as well as other compounds expected in Titan from theoretical modeling, such as other N-organics, and polyynes, first of all C6H2, have never been detected in experimental simulation thus far. All these compounds are thermally unstable, and the temperature conditions used during the simulation experiments were not appropriate. We have recently started a new program of simulation experiments with temperature conditions close to that of Titan's environment. It also uses dedicated analytical techniques and procedures compatible with the analysis of organics only stable at low temperatures, as well solid products of low stability in the presence of O2 and H2O. Spark discharge of N2-CH4 gas mixtures was carried out at low temperature in the range 100-150 K. Products were analysed by FTIR, GC and GC-MS techniques. GC-peaks were identified by their mass spectrum, and, in most cases, by comparison of the retention time and mass spectrum with standard ones. We report here the first detection in Titan simulation experiments of C6H2 and HC5N. Their abundance is a few percent relative to C4H2 and HC3N, respectively. Preliminary data on the solid products indicate an elemental composition corresponding to (H11C11N)n. These results open new prospects in the modeling of Titan's haze making. 相似文献
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M. Cabane P. Coll C. Szopa G. Israël F. Raulin R. Sternberg P. Mahaffy A. Person C. Rodier R. Navarro-Gonzlez H. Niemann D. Harpold W. Brinckerhoff 《Advances in Space Research (includes Cospar's Information Bulletin, Space Research Today)》2004,33(12):2240-2245
Observation of Mars shows signs of a past Earth-like climate, and, in that case, there is no objection to the possible development of life, in the underground or at the surface, as in the terrestrial primitive biosphere. Sample analysis at Mars (SAM) is an experiment which may be proposed for atmospheric, ground and underground in situ measurements. One of its goals is to bring direct or indirect information on the possibility for life to have developed on Mars, and to detect traces of past or present biological activity. With this aim, it focuses on the detection of organic molecules: volatile organics are extracted from the sample by simple heating, whereas refractory molecules are made analyzable (i.e. volatile), using derivatization technique or fragmentation by pyrolysis. Gaseous mixtures thus obtained are analyzed by gas chromatography associated to mass spectrometry. Beyond organics, carbonates and other salts are associated to the dense and moist atmosphere necessary to the development of life, and might have formed and accumulated in some places on Mars. They represent another target for SAM. Heating of the samples allows the analysis of structural gases of these minerals (CO2 from carbonates, etc.), enabling to identify them. We also show, in this paper, that it may be possible to discriminate between abiotic minerals, and minerals (shells, etc.) created by living organisms. 相似文献
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Mai-Julie Nguyen François Raulin Patrice Coll Sylvie Derenne Cyril Szopa Guy Cernogora Guy Israël Jean-Michel Bernard 《Advances in Space Research (includes Cospar's Information Bulletin, Space Research Today)》2008
In the present work, we focused on the possible isotopic fractionation of carbon during the processes involved in the formation of Titan’s tholins. We present the first results obtained on the 12C/13C isotopic ratios measured on Titan’s tholins synthesized in laboratory with cold plasma discharges. Measurements of isotopic ratio 12C/13C, done both on tholins and on the initial gas mixture (N2:CH4 (98:2)) used to produce them, do not show any evident deficit or enrichment in 13C relatively to 12C in the synthesized tholins, compared to the initial gas mixture. This observation allows to go further in the analyses of the ACP experiment data, including part of the Cassini–Huygens mission. 相似文献
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通过激光钎接焊工艺试验,分析了YAG激光加热工艺参数对铝熔体润湿钢表面性能的影响,以激光骑缝束斑加热法验证了6056铝-XC18钢激光搭接钎接焊的可行性. 相似文献
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E Chassefière J-L Bertaux J-J Berthelier M Cabane V Ciarletti G Durry F Forget M Hamelin F Leblanc M Menvielle M Gerasimov O Korablev S Linkin G Managadze A Jambon G Manhès Ph Lognonné P Agrinier P Cartigny D Giardini T Pike W Kofman A Herique P Coll A Person F Costard Ph Sarda Ph Paillou M Chaussidon B Marty F Robert S Maurice M Blanc C d'Uston J-Ch Sabroux J-F Pineau P Rochette 《Advances in Space Research (includes Cospar's Information Bulletin, Space Research Today)》2004,34(8):1702-1709
In view to prepare Mars human exploration, it is necessary to promote and lead, at the international level, a highly interdisciplinary program, involving specialists of geochemistry, geophysics, atmospheric science, space weather, and biology. The goal of this program will be to elaborate concepts of individual instruments, then of integrated instrumental packages, able to collect exhaustive data sets of environmental parameters from future landers and rovers of Mars, and to favour the conditions of their implementation. Such a program is one of the most urgent need for preparing human exploration, in order to develop mitigation strategies aimed at ensuring the safety of human explorers, and minimizing risk for surface operations. A few main areas of investigation may be listed: particle and radiation environment, chemical composition of atmosphere, meteorology, chemical composition of dust, surface and subsurface material, water in the subsurface, physical properties of the soil, search for an hypothesized microbial activity, characterization of radio-electric properties of the Martian ionosphere. Scientists at the origin of the present paper, already involved at a high degree of responsibility in several Mars missions, and actively preparing in situ instrumentation for future landed platforms (Netlander--now cancelled, MSL-09), express their readiness to participate in both ESA/AURORA and NASA programs of Mars human exploration. They think that the formation of a Mars Environment working group at ESA, in the course of the AURORA definition phase, could act positively in favour of the program, by increasing its scientific cross-section and making it still more focused on human exploration. 相似文献