平流层臭氧和辐射场的季节分布特征

利用美国NCAR化学气候耦合模式WACCM3对平流层温度场、风场、臭氧及辐射场进行了模拟.结果表明,在适宜飞艇长期驻留的准零风层高度20～22km(对应大气压强范围为50～30hPa,以下均采用气压值表征对应大气高度),7-8月风速小于5m·s-1的风带可长期稳定在40°N以北.臭氧空间分布显示,在30hPa气压高度处中国地区臭氧浓度出现了带状分布,30hPa高度以下低纬度地区臭氧浓度低于中纬度地区.平流层太阳加热率的时空变化表明,在平流层上层,太阳加热率可达100×10-6K·s-1,而在平流层下层,只有10×10-6K·s-1.6-8月中国区域的太阳加热率大于9月;在100～30hPa高度内,中纬度地区太阳加热率高于低纬度地区,在30hPa高度以上,低纬度地区太阳加热率高于中纬度地区;8-9月30～40hPa高度处,太阳加热率的空间变化较小.在30hPa高度上,太阳加热率在40°N昼夜变化最大;50hPa高度处,太阳加热率的昼夜变化小于30hPa高度处,而且白天太阳加热率出现极大值的纬度明显靠北.平流层低纬度地区的长波加热率小于中纬度地区.青藏高原由于地形特殊,其6-7月的臭氧浓度、太阳加热率和长波加热率均小于同纬度其他地区.      

对流层顶变化对上对流层/下平流层臭氧分布的影响

上对流层和下平流层(UT／LS)，位于8-25km高度之间，是大气中一个很特殊的区域．大部分的臭氧分布在下平流层，在下平流层臭氧的含量发生一个很小的变化，就会对气候和地面的紫外辐射产生很大的影响．而作为气象参数的对流层顶，是充分混合、缺乏臭氧的上对流层和层结稳定、臭氧丰富的下平流层之间的边界或过渡层，其变化对臭氧总量和分布有直接和明显的影响．本文使用二维模式模拟研究对流层顶变化对臭氧在UT／LS分布的影响．模拟结果表明对流层顶的季节变化对UT/LS的臭氧分布有明显的影响，臭氧的局地变化可以超过10％在冬季北半球中纬度对流层顶高度升高1km时，模式结果表明对臭氧分布的影响比较显著，局地变化可超过6％，但是对臭氧总量的影响较小，变化不超过5DU，小于观测资料统计分析的结果。     

The global distribution and variability of stratospheric constituents measured by LIMS

The purpose of the Nimbus 7 LIMS experiment was to sound the composition and structure of the upper atmosphere and provide data for study of photochemistry, radiation, and dynamics processes. Vertical profiles were measured of temperature and ozone (O₃) over the 10-km to 65-km range and water vapor (H₂O), nitrogen dioxide (NO₂), and nitric acid (HNO₃) over the 10-km to ～50-km range. Latitude coverage extended from 64°S to 84°N. Several general features of the atmosphere have emerged from data analyses thus far. Nitrogen dioxide exhibits rapid latitudinal variations in winter and shows hemispheric asymmetry with generally higher vertical column amount in the summer hemisphere. HNO₃ data show that this gas is highly variable with altitude, latitude, and season. Smallest mixing ratios occur in the tropics, and the largest values occur in the high latitude winter hemisphere. The results show that O₃, NO₂, and HNO₃ are strongly affected during a stratospheric warming. There is a persistently low water vapor mixing ratio in the tropical lower stratosphere (～2–3 ppmv), a poleward gradient at all times in the mission, and evidence of increasing mixing ratio with altitude at tropical and middle latitudes.     

Ozone mini-hole observation over the Balkan Peninsula in March 2005

Areas with dimensions of 1000–3000 km in which the total ozone content (TOC) decreases fast are called ozone mini-holes. They are generated mainly dynamically in two ways, either by poor-ozone air mass transport from the tropics to higher latitudes by planetary wave activity or, they are connected with strong adiabatic uplifting of the tropopause height. An ozone mini-hole, generated by the second mechanism, was observed over the Balkan Peninsula on 19/21 March 2005. In the middle of March, the polar vortex was strongly disturbed by Rossby waves, reaching up to the lower stratosphere. Warming episodes over a geographical area, covering the Barents Sea and the Polar Sea north from Central Siberia, displaced a polar vortex fragment extremely southwards. However, the vorticity was weak and the stratospheric temperatures did not reach low values, providing conditions for ozone chemical destruction via heterogenic reactions. At the same time, a Rossby wave ridge was located below the European polar fragment. In the period from 13 to 19 March, the thermal tropopause over Sofia was uplifted almost by 3 km. Ozone distributions observed by the SCIAMACHY instrument on 18–21 March show a fast TOC decrease westwards from Ireland, which was moving eastwards during the next days, increasing the area in which the ozone content decreased. On 20/21 March low ozone content was observed above the Stara Zagora (42°N, 25°E) ground-based station by means of the GASCOD instrument, using DOAS technique. The TOMS Earth probe instrument detected 237 DU over Sofia. This is a record low March value from the beginning of the TOMS instrument measurements in 1978. In March/April the ozone distribution was characterized by its mean annual maximum of 360 DU at 42°N.     

Global structure,seasonal and interannual variability of the eastward propagating tides seen in the SABER/TIMED temperatures (2002–2007)

The present paper is focused on the global spatial (altitude and latitude) structure, seasonal and interannual variability of the most stable in amplitude and phase eastward propagating diurnal and semidiurnal tides with zonal wavenumbers 2 and 3 derived from the SABER/TIMED temperatures for full 6 years (January 2002–December 2007). The tidal results are obtained by an analysis method where the tides (migrating and nonmigrating) and the planetary waves (zonally travelling, zonally symmetric and stationary) are simultaneously extracted from the satellite data. It has been found that the structures of the eastward propagating diurnal tides with zonal wavenumbers 3 and 2 change from antisymmetric with respect to the equator below ∼85 km height, to more symmetric above ∼95 km. The seasonal behavior of the DE3 is dominated by annual variation with maximum in August–September reaching average (2002–2007) amplitude of ∼15 K, while that of the DE2 by semiannual variation with solstice maxima and with average amplitude of ∼8 K. These tides revealed some interannual variability with a period of quasi-2 years. The seasonal behavior of the eastward propagating semidiurnal tide with zonal wavenumber 2 in the southern hemisphere (SH) is dominated by annual variation with maximum in the austral summer (November–January) while that in the northern hemisphere (NH) by semiannual variation with equinoctial maxima. The SE2 maximizes near 115 km height and at latitude of ∼30° reaching an average amplitude of ∼6 K. The seasonal behavior of the eastward propagating semidiurnal tide with zonal wavenumber 3 in both hemispheres indicates a main maximum during June solstice and a secondary one during December solstice. The tide maximizes near 110–115 km height and at a latitude of ∼30° reaching an average amplitude of ∼4.8 K in the SH and ∼4 K in the NH. The tidal structures of the two eastward propagating semidiurnal tides are predominantly antisymmetric about the equator.     

Temperature variability in the tropical mesosphere during the northern hemisphere winter

Temperature observations at 20–90 km height and 5°N–15°N during the period of December 1992–March 1993 from the WINDII and MLS experiments on the UARS satellite are analysed together with MF radar winds and UKMO assimilated fields of temperature and zonal and meridional winds. The correlation between the different datasets at the tropics and zonal mean wind data at mid latitudes is examined for period February–March 1993, when series of stratospheric warming events were observed at middle and high latitudes. Wavelet analysis is applied to investigate coupling between stationary and travelling planetary waves in the stratosphere and the upper mesosphere. Planetary waves m = 1 with periods of 4–7 days, 8–12 days and 13–18 days are found to dominate the period. Westward 7- and 16–18 day waves at the tropics appear enhanced by stationary planetary waves during sudden stratospheric warming events.     

High vertical resolution water vapour profiles in the upper troposphere and lower stratosphere retrieved from MAESTRO solar occultation spectra

An algorithm has been developed that retrieves water vapour profiles in the upper troposphere and lower stratosphere from optical depth spectra obtained by the Measurements of Aerosol Extinction in the Stratosphere and Troposphere Retrieved by Occultation (MAESTRO) instrument onboard the SCISAT satellite as part of the Atmospheric Chemistry Experiment (ACE) mission. The retrieval relies on ro-vibrational absorption of solar radiation by water vapour in the 926–970 nm range. During the iterative inversion process, the optical depth spectra are simulated at the spectral resolution and sampling frequency of MAESTRO using the correlated-k approximation. The Chahine inversion updates the water vapour volume mixing ratio (VMR), adjusting all retrieval layers simultaneously, to match the observed differential optical depth due to absorption by water vapour and ozone at each tangent height. This approach accounts for significant line saturation effects. Profiles are typically obtained from ∼22 km down to the cloud tops or to 5 km, with relative precision as small as 3% in the troposphere. In the lower stratosphere, the precision on water vapour VMR is ∼1.3 μmol/mol in an individual retrieval layer (∼1 km thick). The spectral capability of MAESTRO allows for the clear separation of extinction due to water vapour and aerosol, and for the fitting quality to be quantified and used to determine an altitude-dependent convergence criterion for the retrieval. In the middle troposphere, interhemispheric differences in water vapour VMR are driven by oceanic evaporation whereas in the upper troposphere, deep convection dominates and a strong seasonal cycle is observed at high latitudes.     

Comparison of ozone data derived from SBUV and SAGE with emphasis on longitudinal variations

Stratospheric ozone observations by the SAGE and SBUV satellite instruments in March and April, 1979 have been analyzed. All SAGE profiles have been smoothed vertically over 8 km to provide some compatibility with the SBUV vertical resolution. Comparing the zonal mean ozone mixing ratios against smoothed LIMS profiles, it is inferred that SAGE is systematically overestimating ozone by approximately 20% at tropical latitudes at pressures lower than 5 mb and that SBUV is underestimating ozone by approximately 15% at 50–70° latitude at 10 mb. A comparison of the longitudinal variations of ozone by SBUV and SAGE is made and the detectability of planetary waves in ozone is emphasized. The uncorrelated portion of the SAGE variances are found to be approximately consistent with the SAGE noise model. Based on the correlated variances, the amplitudes of the smoothed SAGE planetary waves in ozone are found to be the same, on average, as in the SBUV experiment at mid-latitudes between 1 and 10 mb. Planetary wave detectability is illustrated during two several day periods at mid-latitudes and a persistent and theoretically-consistent relationship between ozone and temperature is noted. These examples, however, indicate that differences between ozone planetary wave amplitudes derived from the two sensors may occur when there is a strong vertical gradient in wave amplitude.     

Measurements of upper atmosphere wind and temperature from meteorological rocket experiments during winter 1979

This institute conducted a series of meteorological rocket experiments for the upper-atmospheric sounding in the winter of 1979. Within the overlap altitude range with balloon flights, a comparison of the results with the standard radiosonde data indicated that the rocket-borne system was reliable. The measurements from foru rocket flights for the region between 20 and 30 km showed a degree of compatibility to each other while those for above 30 km differed considerably from one another. At low latitude, the temperature profiles in the winter stratosphere in general showed a reasonably good agreement with the U.S. Standard Atmospheric Supplements, 1966 (USSAS 66). A temperature of 2–24°C lower than the USSAS 66, however, was recorded in the lower mesosphere. Above 30 km the maximum diurnal variation in temperature was 9°C or so. In the winter, the wind profile showed the westerlies and the maximum wind velocity of 92.1 Msec^?1 was obtained from these experiments at the height of 60 km.     

FY-3D卫星的北斗掩星分布特征与误差特性

利用2018年1－3月FY-3D卫星的掩星折射率数据,研究了北斗导航卫星系统的掩星分布特点、数据精度以及误差统计特征。北斗导航卫星系统同步静止轨道掩星沿卫星轨道呈弧状分布在南北两极地区,倾斜轨道掩星在东西半球低纬度地区分别形成一小一大两个空洞,中地球轨道掩星则全球均匀分布。北斗掩星折射率数据精度在探测核心区域,即12~32 km范围内,与ERA5再分析资料计算的折射率相比,平均偏差的标准差约为1.5%,在核心区外,标准差从1.5%逐渐增大到6%。静止轨道掩星的平均偏差在高层略大于倾斜轨道和中地球轨道掩星。下降掩星在20 km以上区域的标准差大于上升掩星,20 km以下区域小于上升掩星。高纬地区北斗掩星标准差最小,低纬地区最大,对流层中下层尤其明显。分析结果表明,北斗掩星的数据精度和误差特征与GPS掩星数据相似。      

Vertical wavenumber spectra of atmospheric ozone measured from ozonesonde observations

Vertical profiles of ozone have been measured at balloon altitudes. Our purpose is to examine the character of vertical wavenumber spectra of ozone fluctuations, to assess the possible roles of gravity wave field in ozone fluctuations, and to determine dominant vertical wavelengths of ozone spectra. Vertical wavenumber spectra of 12 ozone fluctuations obtained during June–August 2003 are presented. Results indicate that mean spectral slopes in the wavenumber range from 4.69 × 10⁻⁴ to 2.50 × 10⁻³ cyc/m are about −2.91 in the troposphere and −2.87 in the lower stratosphere, which is close to the slope of −3 predicted by current gravity wave saturation models. The consistency of the observed spectral slopes with the value of −3 predicted by current gravity wave saturation models suggests that the observed ozone fluctuations are due primarily to atmospheric gravity waves. At m = 1/(1000 m) the mean spectral amplitude is over 30 times larger in the lower stratosphere than in the troposphere. Mean vertical wavenumber spectra in area-preserving form reveal dominant vertical wavelengths of ∼2.6 km in the troposphere and ∼2.7 km in the lower stratosphere, which is consistent with the values varying between 1.5 and 3.0 km estimated from the velocity field and temperature field at these heights.     

Recent results on the Venus atmosphere from pioneer Venus radio occultations

Radio occultation measurements of the temperature structure of the Venus atmosphere have been obtained during seven occultation “seasons” extending from December 1978 to December 1983. Approximately 123 vertical profiles of temperature from about 40 km to about 85 km altitudes have been derived. Since these measurements cover latitudes from both poles to the equator, they have shown the latitudinal dependence of thermal structure. There is a smooth transition from the troposphere to the mesosphere at latitudes below about 45°, with the tropopause at about 56 km. The troposphere then rises to about 62 km in the “collar cloud” region between about 60° and 80° latitude, where a strong temperature inversion (up to 30 K) is present. In the polar areas, 80°–90°, the mesosphere becomes isothermal and there is no inversion. This latitudinal behavior is related to the persistent circulation pattern, in which a predominantly zonal retrograde motion at latitudes below 45° gradually changes to a circumpolar vortex at the “collar cloud” latitudes. Indeed, the radio occultation data have been used in a cyclostrophic balance model to derive zonal winds in the Venus atmosphere, which showed a mid-latitude (50°–55°) jet with a speed of about 120–140 ms^?1 at about 70 km altitude /1,2/. The observations obtained in 1983 and 1984 have shown that above the tropopause there is considerable temporal variability in the detailed thermal structure, suggesting that the persistent circulation pattern is subject to weather-like variability.     

A numerical model approximating extreme energetic electron events involved in the physical and chemical processes of the middle atmosphere

Relativistic electrons (with energies >150 keV) which originate in the outer radiation belt and detected by the Russian ‘Meteor’ series of satellites have been correlated with the atmospheric total ozone data compiled by almost 90 stations located around the world within the latitude zone 40°–70°N. In more than 60% of the stations examined we have detected a clear decrease of the ozone 3–5 days after the electron flux excess. A numerical model has been applied to approximate this effect based on relativistic electron initiated nitric oxides creation in the upper mesosphere with subsequent atmospheric transport (both vertical and horizontal) towards the upper stratosphere. A first attempt of local and temporal prediction of ozone depletion because of energetic electrons impact in the middle atmosphere has been illustrated.     

Assessment of the ozone and temperature variability during 1979–1993 with the chemistry-climate model SOCOL

The chemistry-climate model SOCOL has been applied for the study of ozone and temperature anomalies during 1979–1993. Temperature and ozone anomalies have been obtained for a set of model runs forced by all major stratospheric forcing mechanisms. Forcings have been prescribed separately and together to assess their individual influence on stratospheric ozone and temperature. The results of these simulations have been compared to available satellite data. The model captures well ozone depletion and cooling in the upper stratosphere due to increases in the abundance of greenhouse gases and ozone depleting substances in the atmosphere. In the lower stratosphere, the model reproduces the warming over tropical and middle latitudes caused by the El-Chichon and Pinatubo eruptions. However, the simulated ozone response is overestimated in comparison with SAGE data. The best agreement with observations has been obtained for the run with all forcings included. This emphasizes the importance of the volcanic and solar forcings for the correct reproduction of observed trends. Comparison of near-global total ozone anomalies confirms an overestimation of ozone depletion just after volcanic eruptions, while the overall agreement with the model is fairly good.     

On the quasi-biennial oscillation in equatorial stratospheric temperatures and total ozone

The results of a cross-spectral analysis between monthly mean temperatures at 100 mb, 50 mb and 30 mb over the equator and the corresponding monthly mean BUV total ozone at different latitude zones are presented for the period 1970–1977. Significant squared coherences between total ozone and 50 mb equatorial temperatures at 26 months are only found between 5 degrees on each side of the equator, between 45 deg N and 55 deg N and at 45 deg S. At latitudes were the QBO in stratospheric temperature diminishes so does the QBO in total ozone (i.e. close to 35 deg N and 15 deg S). Over subtropical latitudes there is a tendency towards a more biennial oscillation in total ozone (not correlated with the equatorial QBO in stratospheric temperatures) and at 65 deg N and 65 deg S total ozone oscillates at periods greater than the equatorial QBO.     

Temperature comparison between CHAMP radio occultation and TIMED/SABER measurements in the lower stratosphere

Global Positioning System (GPS) receiver on the CHAllenging Mini-satellite Payload (CHAMP) and the Sounding of the Atmosphere using Broadband Emission Radiometry (SABER) instrument, one of four on board the TIMED satellite, provide middle atmosphere temperature profiles by Radio Occultation (RO) and limb viewing infrared emission measurements, respectively. These temperature profiles retrieved by two different techniques in the stratosphere are compared with each other using more than 1300 correlative profiles in March, September and December 2005. The over-all mean differences averaged over 15 and 35 km are approximately −2 K and standard deviation is less than 3 K. Below 20 km of altitude, relatively small mean temperature differences ∼1 K are observed in wide latitudinal range except for June (during the SABER nighttime observation). In the middle to low latitudes, between 30°S and 30°N, the temperature difference increases with height from ∼0–1 K at 15 km, to ∼−4 K at 35 km of altitude. Large temperature differences about −4 to −6 K are observed between 60°S and 30°N and 31–35 km of altitude for all months and between 0° and 30°N below 16 km during June (nighttime).     

Mass spectrometry in the stratosphere

During the last few years a gas expansion system, combined with a mass spectrometer has been developed and successfully flown in the stratosphere. Neutral gas particles are formed into a molecular beam which traverses the ion source of the mass spectrometer without wall interactions. Vertical profiles of constituents such as H₂O, CO₂ and O₃ have been measured in the altitude range of 20 to 40 km during balloon descents. Isotopes of major atmospheric gases (N₂, O₂, Ar) provided in-flight calibration standards.Before each flight the mass spectrometer system was calibrated in the laboratory for many gases of interest, including ozone. Mixing ratios of ozone determined from recent flights have accuracies of better than 5%. The sensitivity of the system was sufficiently high to detect, in addition, the heavy isotope of ozone at mass 50. A pronounced enhancement of heavy ozone in the upper stratosphere has been found. The mass spectrometer system provides the unique opportunity to perform in the stratospherein-situ measurements combined with isotopic studies.     

Latitude gradients in the natural variance in stratospheric conductivity – Implications for studies of long-term changes

Stratospheric electrical conductivity measurements have been made from high altitude research balloons at various locations around the world for more than 40 years. In the stratosphere, conductivity changes may indicate changes in aerosol or water vapor content. In this paper, we will compare the short term variation amplitude in data taken at several latitudes from equatorial to polar cap. Short term variations that occur on time scales of weeks to months (10⁵–10⁷ s) can be attributed to Forbush decreases, geomagnetic storms, aerosol injections by volcanos and forest fires, etc. Variations with time scales of minutes to days (10³–10⁵ s) can have amplitudes of a factor of ∼2 or more at high magnetic latitude. The variance at equatorial latitude is much smaller. The sources of these fluctuations and the latitude gradient remain unknown. Variations of all origins completely obscure any long-term climatic trend in the data taken in the previous four decades at both mid and high latitude.     

Ozone variations observed during the International Ozone Rocket Sonde Intercomparison

The International Ozone Rocket Sonde Intercomparison (IORI) conducted at Wallops Island during October 1979 provided a unique opportunity to observe ozone variations in great detail from several observing systems. The measurement period lasted 15 days during which time ozone observations were taken by ground-based, balloon, rocket, and satellite instruments. These data provided a unique opportunity for diagnosing regional stratospheric variability over a 2 week period. Examination of NMC analyses indicated that during this period the stratospheric polar vortex moved southeastward bringing air from high latitudes to Wallops Island above 10 mb. A concurrent change was observed in the upper stratosphere ozone fields observed by Nimbus-7 SBUV and in the ozone vertical distribution measured by the rocket soundings. In this study the satellite and rocket measurements are compared. The agreement is good, certainly within the errors of the measurements.