SCIAMACHY limb measurements of NO2, BrO and OClO. Retrieval of vertical profiles: Algorithm,first results,sensitivity and comparison studies

The Scanning Imaging Absorption Spectrometer for Atmospheric Chartography (SCIAMACHY) measures scattered sun light also in limb viewing mode (i.e. tangential to Earth’s surface and its atmosphere), which allows determining vertical profiles of atmospheric trace gases. First results on the retrieval of NO₂, BrO and OClO profiles from the SCIAMACHY Limb measurements are presented and compared to independent satellite and balloon borne observations.     

High resolution limb observations of clouds by the CRISTA-NF experiment during the SCOUT-O3 tropical aircraft campaign

The Cryogenic Infrared Spectrometers and Telescopes for the Atmosphere – New Frontiers (CRISTA-NF) experiment on board the Russian research aircraft Geophysica measures limb emission spectra with an unprecedented vertical and horizontal resolution in the 4–15 μm wavelength region. The IR spectra measured during the SCOUT-O3 Tropical Aircraft Campaign have been analysed with respect of cloud occurrence, cloud vertical and horizontal extent, cloud spatial structures and their utilisation for trace gas retrievals. In addition indicators for ice water content and optical thickness of the clouds have been adopted. These new kinds of measurements in the upper troposphere/lower stratosphere region are especially valuable for the design and development of future space borne high resolution limb sounders.     

Radiance calibration of CRISTA-NF

The CRISTA-NF instrument is the airborne version of the CRISTA satellite infrared limb sounder. It has been successfully flown on the Geophysica research airplane during a test campaign in July 2005, during the SCOUT-O3 Tropical Aircraft Campaign in November/December 2005 and during the AMMA campaign in August 2006. Radiance calibrations of the airborne instrument are more complex compared to the satellite instrument because the vacuum shell of CRISTA-NF is confined by a ZnSe (zinc–selenide) window and the detectors can thermally drift during measurement flights. By comprehensive radiance calibrations with a blackbody source the window’s emissivity and transmissivity are determined and the dependence of the instrument sensitivity on the detector temperature is characterized. Taking these effects into account, the remaining radiance error of the calibration is smaller than 3%.