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11.
To better understand the formation of H2O2 in the ozonation of nitrobenzene and its role for the oxidation,a batch reactor of nitrobenzene ozonation was set up.The variables such as pH value,ozone dosage,and the presence of hydroxyl radical scavenger were investigated.The results showed that high accumulations of H2O2 were generally formed at low pH values and low ozone dosages.Moreover,H2O2 mainly formed after nitrobenzene was oxidized by hydroxyl radical during ozonation of the intermediates,such as p-nitrophenol,which reacted with ozone quickly in water.A small amount of additional H2O2 enhanced the nitrobenzene removal slightly.The kinetic study showed that nitrobenzene degradation fitted with pseudo-second-order kinetics well in the experiment.The kinetic constant values correlated linearly with the concentrations of H2O2 added.Thus,it is expected that the H2O2 formed in oxidation of nitrobenzene may initiate ozone decomposition to form hydroxyl radical and finally enhance the degradation of aromatic compounds to a certain extent. 相似文献
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H_∞滤波算法及其在GPS/SINS组合导航系统中的应用 总被引:4,自引:0,他引:4
在对 H∞ 估计问题进行数学描述的基础上,建立了一种 H∞ 次优滤波算法的迭代方程。定性讨论了H∞滤波算法与传统 Kalman滤波器的关系,通过在 GPS/SINS组合系统中的实际应用进一步从精度、鲁棒性等性能指标方面对 H∞ 滤波和 Kalman滤波算法进行了比较。仿真结果表明,在理想条件下,Kalman滤波方法具有较高的精度;但是,当系统模型和外部干扰统计特性发生变化时,H∞ 滤波算法明显具有良好的鲁棒性能,同时,估计精度也较高,有效地克服了 Kalman滤波器存在的局限性。 相似文献
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There is evidence for temperature fluctuations in Planetary Nebulae and in some Galactic H II regions. If such fluctuations occur in the low metallicity, extragalactic H II regions used to probe the primordial helium abundance, the derived 4He mass fraction, YP, could be systematically different from the true primordial value. Although this effect could be large, there are no data which allow us to estimate the size of the temperature fluctuations for the extragalactic H II regions. Therefore, we have explored this effect via Monte Carlo simulations of the data in which the abundances derived from a fiducial data set are modified by T chosen from a distribution with 0 T Tmax where Tmax is varied from 500 K to 4000 K. 相似文献
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双脊矩形管的绕弯成形受内外侧模具的共同约束,不同模具约束下管坯的受力不同,使得其截面变形情况也不相同,而截面变形严重地影响弯管件的成形质量和使用性能。因此,基于ABAQUS有限元平台建立了双脊矩形管E弯成形三维有限元模型,并通过实验验证了模型的可靠性。采用所建模型,研究了内外侧模具约束条件对双脊矩形管E弯截面变形的影响规律,发现当只有内腹板脊槽受约束时,内腹板脊槽的内缩变形可得到较好的控制,而其他部位的变形则有增大的趋势;当只有外腹板脊槽受约束时,内腹板脊槽宽度变形基本不发生变化,而其他部位的变形则有减小的趋势;当内外腹板脊槽均受约束时,可较好地控制双脊矩形管E弯过程中的截面变形。芯头个数对整管截面高度、宽度、外腹板脊槽宽度与两脊槽底部的间距的变形影响较大,但对内腹板脊槽宽度的变形影响不显著。 相似文献
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M. Prabhu K. Unnikrishnan 《Advances in Space Research (includes Cospar's Information Bulletin, Space Research Today)》2018,61(7):1672-1688
In the present work, we analyzed the daytime vertical E × B drift velocities obtained from Jicamarca Unattended Long-term Ionosphere Atmosphere (JULIA) radar and ΔH component of geomagnetic field measured as the difference between the magnitudes of the horizontal (H) components between two magnetometers deployed at two different locations Jicamarca, and Piura in Peru for 22 geomagnetically disturbed events in which either SC has occurred or Dstmax < ?50 nT during the period 2006–2011. The ΔH component of geomagnetic field is measured as the differences in the magnitudes of horizontal H component between magnetometer placed directly on the magnetic equator and one displaced 6–9° away. It will provide a direct measure of the daytime electrojet current, due to the eastward electric field. This will in turn gives the magnitude of vertical E × B drift velocity in the F region. A positive correlation exists between peak values of daytime vertical E × B drift velocity and peak value of ΔH for the three consecutive days of the events. It was observed that 45% of the events have daytime vertical E × B drift velocity peak in the magnitude range 10–20 m/s and 20–30 m/s and 20% have peak ΔH in the magnitude range 50–60 nT and 80–90 nT. It was observed that the time of occurrence of the peak value of both the vertical E × B drift velocity and the ΔH have a maximum (40%) probability in the same time range 11:00–13:00 LT. We also investigated the correlation between E × B drift velocity and Dst index and the correlation between delta H and Dst index. A strong positive correlation is found between E × B drift and Dst index as well as between delta H and Dst Index. Three different techniques of data analysis – linear, polynomial (order 2), and polynomial (order 3) regression analysis were considered. The regression parameters in all the three cases were calculated using the Least Square Method (LSM), using the daytime vertical E × B drift velocity and ΔH. A formula was developed which indicates the relationship between daytime vertical E × B drift velocity and ΔH, for the disturbed periods. The E × B drift velocity was then evaluated using the formulae thus found for the three regression analysis and validated for the ‘disturbed periods’ of 3 selected events. The E × B drift velocities estimated by the three regression analysis have a fairly good agreement with JULIA radar observed values under different seasons and solar activity conditions. Root Mean Square (RMS) errors calculated for each case suggest that polynomial (order 3) regression analysis provides a better agreement with the observations from among the three. 相似文献
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