Improvement of flight hardware and isothermal Marangoni convection under micro-gravity conditions

During parabolic flights three different kinds of experiments were performed under reduced gravity conditions. The experiments were: I. A general learning process to work with hardware and fluid under micro-gravity conditions. II. The investigation of critical parts of hardware or critical moments in experiments. This can be a part in the preparation of future sounding rocket or Spacelab flights. III. The possibility to perform scientific experiments under micro-gravity conditions within 22 seconds. In the joined parabolic flights of march 1986 the main interest was to perform experiments with Marangoni convection due to concentration gradients along the gas-liquid interface under isothermal conditions. One experiment was performed with a horizontal surface tension gradient and the other observed Marangoni convection was due to the evaporation of a component from a solution under steady state conditions.     

天舟一号货运飞船空间实验装置蒸发相变地面实验

以天舟一号货运飞船为依托,开展空间蒸发相变传热规律的科学实验研究,探索重力对蒸发传热传质过程的影响规律.设计了一套地面蒸发实验平台,以蒸发相变液体FC-72为研究对象,通过红外热像仪测温、热流量计、差分热电偶等手段,观测FC-72液层在不同台面温度、注液量等情况下的相变界面变化、蒸发表面特性、流体物性及Marangoni对流涡胞的变化等,获取其蒸发两相流体的液层温度差、表面温度场、热流量值、蒸发速率和涡胞结构等.实验结果表明:在其他条件不变的情况下,FC-72液层与蒸发台面的温差越高,其蒸发速率越快;注液量越大,蒸发速率也越大;在蒸发过程中出现了浮力对流涡胞和Marangoni对流涡胞.此外,通过地面蒸发实验可以确定空间科学实验选用的实验介质和材料,进而优化确定空间科学实验的工况、参数及流程等,部分地面实验结果也将直接成为天地对比实验的科学成果.      

微重力环境下蒸发液层热毛细对流的数值模拟

提出了一种新模型来研究由单一物质构成的液层在其纯蒸气中的蒸发.液层置于微重力环境中并且受到水平方向温度梯度的作用,液层的热毛细对流和蒸发耦合在一起,使得气液界面的传热传质规律更加复杂.用理论分析的方法求解了不考虑热毛细效应的纯蒸发模型,得出温度场分布和界面质量流量的解析表达式.对于热毛细对流和蒸发耦合情况,采用有限差分的投影算法同时求解Navier-Stokes方程和能量方程,得到了不同蒸发Biot数和Marangoni数下流场和温度场的稳态数值解.论述了蒸发Biot数和Marangoni数对界面传热传质的影响,提出并解释了蒸发和热毛细对流耦合的三种模式.      

Convective stability of immiscible fluids in parallel shearing motion —role of the diffusion

Coupling between the Laplace and the Marangoni effects in a parallelly moving diffusion system is studied. Convective instability arises from either pure Marangoni effect or Laplace effect which is always influenced by the Marangoni contribution. Near to , a common stable region is found under disturbances of concentrations and micro interface deformations. Gravity plays a role through the Laplace condition.     

过冷核态池沸腾中的Marangoni效应

分析了过冷核态池沸腾过程中气泡横向运动现象,指出其成因在于相邻气泡界面温度差引起的Mara-ngoni对流对周围液体的吸引.通过对该流动的尺度分析,得到了气泡横向运动特征速度及其可观测度的估算公式,其预测结果与实验观测相一致.特别是对极细小的初始核化气泡,该公式预测了强烈的横向Marangoni对流会导致气泡顶端微射流的形成.该效应在加热面水平向下或微重力沸腾等气泡脱落频率较低的情形中尤为重要.      

Oscillatory thermocapillary convection in floating zones under normal- and micro-gravity

The thermocapillary convection in a floating zone becomes oscillatory, exceeding a Marangoni number of approximately 10⁴. The oscillatory state of thermocapillary convection has been verified under 1 g and 10^?4 g and the features seem to be fairly independent of the gravity level. The transition point from the laminar to the oscillatory state (critical Marangoni number), however, depends on the magnitude and direction of the buoyant force.     

Recent development of Marangoni flows theory and experimental results

Microgravity fluid dynamics deals with the thermodynamics and dynamics of fluid systems in low-gravity environments and, thus, covers a rather large variety of subjects /1/. Among them, free convection in systems with fluid-fluid interfaces has received renewed attention because these systems are found in many materials sciences processes and exhibit a number of new, interesting phenomena. This paper surveys some recent studies by the author and his coworkers on the free convection occurring in a system of two interfacing, immiscible fluids subject to an imposed temperature gradient in a gravity environment. In such a system, three classes of free convection may be distinguished: natural, Marangoni, and combined free convection, according to whether it is caused by thermally induced buoyant forces, Marangoni stresses, or both. For each class one may further distinguish different regimes according to the relative importance of convective and diffusive transport of momentum and internal energy.First, the use of order of magnitude analysis is illustrated to identify and determine the types of flow regimes that can be established for each class of free convection. Subsequently, the attention is focused on the study of the main features of the two classes of flow regimes that can be established when the leading driving action is the Marangoni stress: Marangoni boundary layers and Marangoni-Stokes flow. Finally, a brief review of the experimental experience of the author's team is reported, looking in particular at the space experiments performed on board the missions SL1 and D1 of the Spacelab.     

实践十号卫星蒸发对流箱地面科学实验结果分析

实践十号卫星蒸发对流实验旨在研究置于加热底板的蒸发液滴在相变过程中,表面蒸发与表面张力驱动对流的耦合机理及其不稳定性.为与空间实验结果进行对比,利用蒸发对流箱完成在轨工况的科学匹配实验,获得相应工况的地面科学数据、工程参数及实验图像.通过对地面科学匹配实验结果进行分析,得到不同工况下液滴形貌（体积、表面积、接触角、液滴高度、液滴直径）变化规律,以及液滴蒸发过程中温度、热流量、蒸发速率和蒸发流量的变化规律.依据实验结果分析研究了具有质量交换的复杂流体相变界面的热质传输规律.      

Marangoni convection in a liquid layer under the simultaneous action of a transverse magnetic field and rotation

Asymptotic stability characteristics with respect to the onset of Marangoni convection in a liquid layer under the simultaneous action of a large transverse magnetic field and a large rate of rotation are investigated. In certain parameter ranges there is a decrease in critical Marangoni number for increasing magnetic field and rotation depending on the coupling between interfacial perturbations and rotation.     

A sounding rocket experiment on the marangoni convection

During a 6-minutes free flight of a sounding rocket an experiment on the thermal Marangoni convection in a right circular cylindric floating zone was carried out to verify the thermal Marangoni convection by flow visualisation for the first time at 10^?4 g. From the motion picture analysis the velocity distributions are obtained. The interdependence between the two velocity maxima and the S-shaped temperature distribution on the free surface is discussed. The influence of the heat transfer caused by the flow of the surrounding air induced by the thermal Marangoni convection itself is considered briefly.     

Two-dimensional convection in liquid layer related to crystal growth techniques in space

In this paper, the Marangoni convection including buoyancy convection in two-dimensional fluid model was investigated experimentally and theoretically. The transparent liquid in the test cell was heated and cooled under various conditions. The fluid flow driven by surface tension and by buoyancy force was visualized and measured. The flow patterns, velocity distributions and temperature field were obtained and they were compared with the results of the numerical solutions. The effect of the configuration and the convection in microgravity on crystal growth was discussed. The temperature field of the crystallizing surface was predicted.     

Study of the Marangoni convection around a surface tension minimum under microgravity conditions

At equilibrium, aqueous fatty alcohol solutions presents a surface tension minimum versus temperature. The influence of such an extremum on the Marangoni convection is studied. Two experiments have been performed under microgravity conditions (Texus 8 (1983) and Texus 9 (1984) flights). The velocity fields are determined by following the paths of tracer particles and furthermore, in the Texus 9 experiment, differential interferograms have been recorded.     

Microgravity experiments on the transition from laminar to oscillatory thermocapillary convection in floating zones

The onset of oscillatory thermocapillary convection in floating zones has been measured under microgravity in two sounding rocket experiments TEXUS and on board of the satellite SPAS-01. We report on the critical Marangoni numbers measured under μ-g and in the 1-g reference experiments     

Thermocapillary-driven convection in supported and floating-zone crystallization

Marangoni flow was induced in a thin disk of molten tin with an atomically clean surface by heating it from below in an ultra high vacuum apparatus. The radial distribution of temperature was measured and no temperature oscillations were observed. Strong mechanical disturbances introduced at a Marangoni number of about 4300 died out quickly with time indicating that the system was stable. Mathematical models indicate that strong flows in a two cell structure exist under the conditions studied, and that the velocity profile in the cell near the surface is of the bouindary layer type which varies rapidly with depth.     

环形浅液池内低Prandtl数流体超临界热毛细对流演化

为研究低Prandtl数（Pr）流体热毛细对流演化过程，对环形浅液池内Pr=0.011的流体热毛细对流进行三维数值模拟.研究发现:当Marangoni数较小时，流动为轴对称稳态流动；当Marangoni数超过某一临界值后，流动失稳并转变为热流体波，其波数随Marangoni数增加而减小，而波动主频增大；随着Marangoni数增加，流动加强，沿周向运动的热流体波演变为沿径向运动的径向波，其波数大大减小；当Marangoni数继续增加时，波动频谱曲线噪声增加，呈广谱特性.因此，在计算范围内热毛细对流的演化过程为:轴对称稳态流动-热流体波-单周期径向波-多周期三维振荡流动.      

Direct observation of processes in a solidifying dispersion

The evolution of a dispersion under the action of temperature gradients and solidification was followed optically in a transparent molten salt (CsCl) with inclusions of Pb-droplets and gas bubbles. This system is believed to model a solidifying metallic alloy. Rejection of Pb-particles by the solidification front was observed, while large gas bubbles were incorporated. Thermocapillary convection at the gas bubbles considerably distorted the temperature field and even caused local remelting. Marangoni migration of bubbles was not observed, contrary to expectations.     

蒸发效应与热毛细对流耦合现象的实验研究

实验研究了矩形液池中蒸发薄液居中蒸发效应与热毛细对流的耦合机理. 对于单纯的热毛细对流稳定性从实验和理论上已有深入研究,但目前国际上对带有菇发界面的热毛细对流问题尚缺乏研究. 特别是近来的研究发现,气液界面的蒸发对热毛细对流稳定性有很大的影响. 本实验以温度为主要控制参数,测量了不同工况下蒸发界面不同点的蒸发速率和表层温度,并利用 PIV 方法分析得到了液体内的嘛场分布. 实验结果发现,随着沿界面的温差增加,蒸发液体内的流型从稳定的单涡胞结构变为稳定的多祸胞结构,并最终演变为紊流结构. 综合分析以上测量结果并与理论分析结果进行了比较。      

Onset of Marangoni convection in an infinite layer of an electrically conducting liquid under magnetic field

The onset of Marangoni convection in an electrically conducting liquid is studied theoretically for the case that the liquid is subjected to a vertical temperature gradient and a magnetic field with arbitrary orientation.The effects of the intensity of magnetic field, the angle of inclination of magnetic field and the Biot number at the free surface on both the critical Marangoni number and the flow pattern are made clear.     

Marangoni effects under electric fields

An electric field when applied across liquid-liquid interface was found to cause, due to different susceptibilities of the two phases, what the authors would term as Marangoni “type” of instabilities, that resulted in the generation of bubbles/drops and caused the movement of the interface countering gravity. Thus “mixing” of the two phases would occur and in systems involving mass transfer, enhanced rates of transfer could be expected.Equations for the bubble formation involving parameters such as electrostatic pressure, surface tension, gravity force have been derived.In the case of non-gravitational or weak-gravitational fields such as obtainable in space, the separation of two liquids one below the other, as obtaining on the earth, exhibiting an interface may well nearly be impossible. Under such conditions recourse may have to be taken to super-imposition of other fields as a tool for obtaining the necessary contacting/separation. The dynamics of bubble formation etc. under these contexts are theoretically analysed.     

Conditions for the onset of temperature oscillations in a simulated floating-zone configuration

The floating-zone method for crystal growth is studied in simulated low-gravity conditions by suspending a drop of fluid vertically between two circular rods and heating the upper rod with a heater. Flow and temperature oscillations are observed under certain conditions. The temperature oscillation level and the oscillation frequency are measured against the Marangoni number for several aspect ratios using hexadecane and Fluorinert as the test fluids. It is observed that, contrary to what has been believed, the Marangoni number is not the proper parameter to describe the onset of oscillation.