Most suitable conditions for aerosol monitoring from space

Numerical modelling is used to search for the most suitable conditions, with the object of determining the atmospheric turbidity (aerosol optical depth) from upward emerging spectral radiances in cloudfree pixels over water surfaces. The most suitable conditions are those where the influence of the turbidity on the radiance most strongly outweighs that of the other optically acting constituents. Since the actual values of these constituents of atmosphere and surface are usually known only within certain limits, using the most suitable conditions minimizes the uncertainty in the turbidity to be derived from satellite measurements. As a result, favorable zenith angles of the satellite and favorable wavelengths are presented for an atmosphere with maritime aerosols with and without Saharan dust. The results represent an advance on a paper published by the authors in 1981 [1].     

Interpretation of data on laser sensing of aerosol atmosphere from space

A single-frequency lidar, using aerosol scattering as an informative component, is the simplest and reliable facility for remote sensing of the atmosphere. The information on vertical distribution of atmospheric aerosol which can be obtained using such a lidar is necessary for investigating the physics of atmospheric processes and forecast of optical state of the atmosphere. At the same time, the interpretation of data on single-frequency sounding is associated with some difficulties of fundamental character, mainly due to insufficient software of the experiment. Under such conditions the problems of optimal processing of lidar returns aiming at extracting the useful information on aerosol are of great importance, especially if one takes into account the hindering effects of atmospheric background and optical noises. This paper presents a statistical approach to this problem, and the possibilities of single-frequency sounding from space are analyzed.     

The role of aerosols in the climate system: Results of numerical experiments in climate models

Three principal questions are recurrent with the consideration of an aerosol related climatic effect: (1) do aerosols heat or cool the atmosphere, (2) are aerosol climatic effects significant and (3) can numerical models be validated by predicting a climatic change associated with a measured aerosol-event. Each of these questions will be addressed from a historical perspective. In addition, the most recent aerosol-related modeling will be discussed as well as recommendations for future research.     

Detection of aerosol pollution sources during sandstorms in Northwestern China using remote sensed and model simulated data

The present paper has used a comprehensive approach to study atmosphere pollution sources including the study of vertical distribution characteristics, the epicenters of occurrence and transport of atmospheric aerosol in North-West China under intensive dust storm registered in all cities of the region in April 2014. To achieve this goal, the remote sensing data using Moderate Resolution Imaging Spectroradiometer satellite (MODIS) as well as model-simulated data, were used, which facilitate tracking the sources, routes, and spatial extent of dust storms. The results of the study have shown strong territory pollution with aerosol during sandstorm. According to ground-based air quality monitoring stations data, concentrations of PM₁₀ and PM_2.5 exceeded 400?μg/m³ and 150?μg/m³, respectively, the ratio PM_2.5/PM₁₀ being within the range of 0.123–0.661. According to MODIS/Terra Collection 6 Level-2 aerosol products data and the Deep Blue algorithm data, the aerosol optical depth (AOD) at 550?nm in the pollution epicenter was within 0.75–1. The vertical distribution of aerosols indicates that the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) 532?nm total attenuates backscatter coefficient ranges from 0.01 to 0.0001?km^?1?×?sr^?1 with the distribution of the main types of aerosols in the troposphere of the region within 0–12.5?km, where the most severe aerosol contamination is observed in the lower troposphere (at 3–6?km). According to satellite sounding and model-simulated data, the sources of pollution are the deserted regions of Northern and Northwestern China.     

Evaluation and utilization of CloudSat and CALIPSO data to analyze the impact of dust aerosol on the microphysical properties of cirrus over the Tibetan Plateau

The present study elucidates on the evaluation of two versions (V3 and V4.10) of vertical feature mask (VFM) and aerosol sub-types data derived from the Cloud-Aerosol LiDAR and Infrared Pathfinder Satellite Observations (CALIPSO), and its utilization to analyze the impact of dust aerosol on the microphysical properties of cirrus over the Tibetan Plateau (TP). In conjunction to the CALIPSO, we have also used the CloudSat data to study the same during the summer season for the years 2007–2010 over the study area 25–40°N and 75–100°E. Compared to V3 of CALIPSO, V4.10 was found to have undergone substantial changes in the code, algorithm, and data products. Intercomparison of both versions of data products in the selected grid between 30–31°N and 83–84°E within the study area during 2007–2017 revealed that the VFM and aerosol sub-types are in good agreement of ～95.27% and ～82.80%, respectively. Dusty cirrus is defined as the clouds mixed with dust aerosols or existing in dust aerosol conditions, while the pure cirrus is that in a dust-free environment. The obtained results illustrated that the various microphysical properties of cirrus, namely ice water content (IWC), ice water path (IWP), ice distribution width (IDW), ice effective radius (IER), and ice number concentration (INC) noticed a decrease of 17%, 18%, 4%, 19%, and 10%, respectively due to the existence of dust aerosol, consistent with the classical “Twomey effect” for liquid clouds. Moreover, the aerosol optical depth (AOD) showed moderate negative correlations between ?0.4 and ?0.6 with the microphysical characteristics of cirrus. As our future studies, in addition to the present work undertaken, we planned to gain knowledge and interested to explore the impact of a variety of aerosols apart from the dust aerosol on the microphysical properties of cirrus in different regions of China.     

Investigation of the atmospheric aerosols by the visible and IR channels of the AVHRR radiometer on NOAA-6

The diffusely reflected radiation in the daytime and diffusely transmitted radiation at night from an inhomogeneous, plane parallel planetary atmosphere bounded by the ocean surface was calculated at the visible and IR region. In the daytime the effect of the solar radiation from top was taken into account. The present study has dealt with the problem of no cloud contamination in data. In the atmosphere, water vapor, molecular nitrogen, nitrous oxide, carbon dioxide and methane as absorbent constituents and aerosols as the scattering constituent were taken into account. The ocean surface as a lower boundary was simulated by many facets whose slopes are according to the isotropic Gaussian distribution [1]. It was found that it is suitable for deriving the total optical thickness in the direction of about 15 degrees away from the specular direction at 3.7μm in the daytime, with the aid of visible region of spectrum [2]. As for sea surface temperature, for a sample analysis, derived SST was within the accuracy of 1–2K at the center of the sun glint and within the accuracy of 0.5K in the rest of the region at 3.7μm in the daytime, Furthermore computational results suggest that the comparison of temperature in the daytime with that at night at 3.7μm make it possible to separate the effect of aerosols from the total optical thickness. Thus it was found from the computations that with the aid of daytime and night time data, it is possible to derive the atmospheric water vapor, aerosols and sea surface temperature simultaneously.     

A comparison of atmospheric aerosol measurements by various satellite sensors

Investigations to measure the vertical optical thickness of aerosols over ocean surfaces has been conducted using several different satellite sensors. Landsat 1 and Landsat 2 data originally confirmed that a linear relationship exists between the upwelling visible radiance and the aerosol optical thickness (about 90% of this thickness is generally in the lowest 3 km of the atmosphere). Similar relationships have also been found for sensors on GOES-1, SMS-2, NOAA-5, and NOAA-6 satellites. The linear relationship has been shown theoretically to vary with the aerosol properties, such as size distribution and refractive index, although the Landsat data obtained at San Diego showed little variability in the relationship. The differences between the results found for the various satellite sensors are discussed, and are attributed mainly to uncertainties in the calibration of the sensors. To investigate the general applicability of the technique to different locations, a global-scale ground truth experiment was conducted with the AVHRR sensor on NOAA-6 to determine the relationship at eleven ocean sites around the globe. Analysis of the data shows good agreement between the satellite and ground truth values of the aerosol optical thickness, and indicates that the technique has global application. At two of the sites, multispectral radiometric measurements of the Junge aerosol size distribution parameter were made, and showed good agreement with a value inferred from the AVHRR Channels 1 and 2 radiances.     

Optical properties of dust and the opacity of the Martian atmosphere

Particulate component of the Mars atmosphere composed by micron-sized products of soil weathering and water ice clouds strongly affects the current climate of the planet. In the absence of a dust storm so-called permanent dust haze with τ ≈ 0.2 in the atmosphere of Mars determines its thermal structure. Dust loading varies substantially with the season and geographic location, and only the data of mapping instruments are adequate to characterize it, such as TES/MGS and IRTM/Viking. In spite of vast domain of collected data, no model is now capable to explain all observed spectral features of dust aerosol. Several mineralogical and microphysical models of the atmospheric dust have been proposed but they cannot explain the pronounced systematic differences between the IR data (τ = 0.05–0.2) and measurements from the surface (Viking landers, Pathfinder) which give the typical “clear” optical depth of τ ≈ 0.5 from one side, and ground-based observations in the UV–visible range showing much more transparent atmosphere, on the other side. Also the relationship between τ₉ and the visible optical depth is not well constrained experimentally so far. Future focused measurements are therefore necessary to study Martian aerosol.     

The MAGO experiment for dust environment monitoring on the Martian surface

Among the main directions identified for future Martian exploration, the study of the properties of dust dispersed in the atmosphere, its cycle and the impact on climate are considered of primary relevance. Dust storms, dust devils and the dust “cycle” have been identified and studied by past remote and in situ experiments, but little quantitative information is available on these processes, so far. The airborne dust contributes to the determination of the dynamic and thermodynamic evolution of the atmosphere, including the large-scale circulation processes and its impact on the climate of Mars. Moreover, aeolian erosion, redistribution of dust on the surface and weathering processes are mostly known only qualitatively. In order to improve our knowledge of the airborne dust evolution and other atmospheric processes, it is mandatory to measure the amount, mass-size distribution and dynamical properties of solid particles in the Martian atmosphere as a function of time. In this context, there is clearly a need for the implementation of experiments dedicated to study directly atmospheric dust. The Martian atmospheric grain observer (MAGO) experiment is aimed at providing direct quantitative measurements of mass and size distributions of dust particles, a goal that has never been fully achieved so far. The instrument design combines three types of sensors to monitor in situ the dust mass flux (micro balance system, MBS) and single grain properties (grain detection system, GDS + impact sensor, IS). Technical solutions and science capabilities are discussed in this paper.     

气溶胶光学特性偏振遥感反演算法

陆地上空大气顶的辐射主要由大气散射和地表反射组成,一般地表反射的贡献要大于大气散射的贡献,使得陆地上空气溶胶的特性提取非常困难,而偏振信息只强烈依赖于散射粒子的特性,发展基于偏振信息的气溶胶反演方法是非常有效的. 通过对矢量辐射传输方程求解进行研究,基于倍加累加法矢量辐射传输模式分析影响气溶胶反演的主要因素,确定多维参数查找表建立方法,利用POLDER(Polarization and Directionality of the Earth-s Reflectances)提供的反射率和偏振反射率数据,发展了一种利用反射率和偏振反射率查找表迭代查找反演气溶胶光学参数和地表反射率的算法,实现了对北京、香河、Dalanzadgad观测站上空气溶胶光学厚度、粒子半径、折射指数和地表反射率的反演.用AERONET(Aerosol Robotic Network)地基数据对反演结果进行了验证.     

New insights into Titan's organic chemistry in the gas and aerosol phases.

Titan, the largest satellite of Saturn, with a dense atmosphere very rich in organics, and many couplings in the various parts of its "geofluid", is a reference for studying prebiotic chemistry on a planetary scale. New data have been obtained from experiments simulating this organic chemistry (gas and aerosol phases), within the right ranges of temperature and a careful avoiding of any chemical contamination. They show a very good agreement with the observational data, demonstrating for the first time the formation of all the organic species already detected in Titan atmosphere including, at last, C4N2, together with many other species not yet detected in Titan. This strongly suggests the presence of more complex organics in Titan's atmosphere and surface, including high molecular weight polyynes and cyanopolyynes. The NASA-ESA Cassini-Huygens mission has been successfully launched in October 1997. The Cassini spacecraft will reach the Saturn system in 2004 and become an orbiter around Saturn, while the Huygens probe will penetrate into Titan's atmosphere. In situ measurements, in particular from Huygens GC-MS and ACP instruments, will provide a detailed analysis of the organics present in the air, aerosols, and surface. This very ambitious mission should yield much information of crucial importance for our knowledge of the complexity of Titan's chemistry, and, more generally for the field of exobiology.     

Satellite measurements of tropospheric aerosols

The ability to measure tropospheric aerosols over ocean surfaces has been demonstrated using several different satellite sensors. Landsat data originally showed that a linear relationship exists between the upwelling visible radiance and the aerosol optical thickness (about 90% of this thickness is generally in the lowest 3 km of the atmosphere). Similar relationships have also been found for sensors on GOES, NOAA-5 and NOAA-6 satellites. The linear relationship has been shown theoretically to vary with the aerosol properties, such as size distribution and refractive index, although the Landsat data obtained at San Diego showed little variability in the relationship. To investigate the general applicability of the technique to different locations, a global-scale ground-truth experiment was conducted in 1980 with the AVHRR sensor on NOAA-6 to determine the relationship at ten ocean sites around the globe. The data for four sites have been analyzed, and show excellent agreement between the aerosol content measured by the AVHRR and by sunphotometers at San Diego, Sable Island and San Juan, but at Barbados, the AVHRR appears to overestimate the aerosol content. The reason for the different relationship at the Barbados site has not been definitely established, but is most likely related to problems in interpreting the sunphotometer data rather than to a real overestimation by the AVHRR. A preliminary analysis of AVHRR Channel 1 (0.65 μm) and Channel 2 (0.85 μm) radiances suggest that useful information on the aerosol size distribution may also be obtained from satellite observations.     

Atmospheric electrical conductivity measurements and modeling for application to air pollution studies

The experimentally measured ground level atmospheric electrical conductivity is validated from a simplified ion–aerosol model for which the inputs are ionization rate from surface radioactivity, aerosol density and meteorological parameters. Also estimated from the model is the reduction in conductivity for assumed aerosol levels. It is seen that for an increase of ambient aerosols by threefold the percent reduction in conductivity is 7% and it is 10% for an increase by sixfold. Thus, the variations in the measured ground level conductivity can be used to examine the atmospheric pollution, if any.     

星载FPI探测低热层温度的研究

80～350km高度区域的大气温度与风场探测研究对于认识全球性空间动力学和日地耦合机制具有重要科学意义.法布里-珀罗干涉仪(FPI)能够通过分析接收光的干涉环反演计算出一定高度大气层的风场和温度.近年来,中国利用多种地基探测设备对中高层大气进行了观测研究,对于温度反演和星载探测技术的研究开始起步.本文基于系统传输函数和发射谱线函数的卷积,讨论了利用FPI探测高空大气温度反演计算的原理;分析了星载FPI探测的方法,根据星载FPI探测与地基探测的不同点,仿真了星载探测干涉图;结合中国观测技术现况及空间探测需要,讨论了发展星载空间环境探测仪的可行性.      

The physical mechanism of the solar variability influence on electrical and climatic characteristics of the troposphere

Possible mechanisms of solar–climatic connections, which may be of importance over short and long time intervals, are discussed. The variations of energetic balance of Earth’s climatic system for the last 50 years are estimated. It is ascertained that the imbalance between the flux of solar energy that comes to the Earth and radiates to space is of 0.1% for the last ten years. The significance is analyzed for the possible influence of variations of solar constant upon the energetic balance of the atmosphere.The physical mechanism of the influence of solar activity on climatic characteristics and the atmospheric circulation is suggested and theoretically substantiated. The mechanism is based on the redistribution in lower-troposphere of condensation nuclei by the vertical electric field. This electric field is determined by the ionosphere–Earth electric potential, which in the Polar Regions is controlled not only by tropical thunderstorms and by the galactic cosmic-ray intensity but also by solar cosmic-ray fluxes. The height redistribution in the atmosphere of condensation nuclei with a change of the electric field of the atmosphere is accompanied by a change in total latent heat (phase transition of water vapor), by changes in radiation balance, and by subsequent changes of the thermobaric field of troposphere. The results of analysis of thermobaric field variations for the periods of invasion of abnormally powerful solar cosmic ray fluxes and magnetic storms confirm the reality of manifestation of heliogeophysical disturbances.     

Is there an abnormal enhancement of atmospheric aerosol before the 2008 Wenchuan earthquake?

There are extensive reports of ionospheric disturbances before the great 2008 Wenchuan earthquake, which are possibly explained by seismogenic electric field hypotheses linked with the aerosols injected in atmosphere. This paper attempts to investigate the possible change of atmospheric aerosol optical depth (AOD) associated with this earthquake by using MODIS data from both Terra and Aqua satellites. The result shows a clear enhancement of AOD along the Longmenshan faults 7 days before the quake, which is 1 day and 4 days earlier than the reported negative and positive ionospheric disturbances, respectively, and is 1 day earlier than or quasi-synchronism with other reported atmospheric anomalies including air temperature, outgoing longwave radiation and relative humidity. Particularly, the spatial distribution of AOD enhancement is very local and it is correlated well with the active faults and surface ruptures. We suggest that this unique enhancement could be associated with the Lithosphere–Atmosphere–Ionosphere coupling process during the preparation of the Wenchuan earthquake.     

火星信道衰落特性对通信链路预算的影响

对火星星体段的信道衰落特性进行研究.通过对近火段自然环境因素的分析,提取影响火星通信性能的因素,重点分析火星的大气、云雾、沙尘对通信信道的衰落作用机理;并以NASA实际火星探测任务为例,针对以上衰落因素对UHF,S,X和Ka频段下的通信链路影响情况进行仿真;结合实际探测数据对地球通信链路预算模型进行修正,提出一种适用于火星通信链路预算的模型;明确火星大气衰落、云雾衰落、沙尘衰落的取值范围.研究结果可作为火星及其他深空探测任务的通信系统设计与链路复核复算的参考.      

Preliminary calibration results of VEGA 1 and 2 SIGMA-3 gas chromatograph

SIGMA - 3 gas chromatograph on board VEGA 1 and 2 landing probes has been operated successfully in the 60 - 50 km altitude range, providing several in - situ chemical analysis of the gas and the aerosols of Venus cloud layers. Post flight calibration required to derive atmospheric abundancies from gas chromatograms were carried out using the SIGMA - 3 spare model. A Venus atmospheric aerosol simulation chamber was used in which sulfuric acid droplets were generated. Preliminary results of these calibration experiments indicate that the concentration of sulfuric acid in the upper part of the clouds ( 60 to 55 km) is about 1 mg/m³ and suggest that an additional constituant must be present in noticeable amount in the aerosols. From these experiments the mixing ratio upper limits of SO₂ is 100 ppmV and of H₂S and COS is few 10 ppmV.     

Plan for the implementation of the world climate research programme

The objectives of the World Climate Research Programme (WCRP) are expressed in terms of increasing time scales, from several weeks to several decades. The Programme calls for substantial developments in modelling the interaction of the global atmosphere with the ocean, land surface and sea-ice, as well as improved computations of radiation transfer in the presence of clouds, aerosols and absorbing gases. These developments require a large variety of space as well as surface based observations, and especially, additional efforts for systematic processing of available data to produce consistent records of significant climatological variables. The forthcoming development of a new generation of ocean observing satellites will be an essential component of the WCRP, as they will provide the data base for the large-scale oceanographic projects, the World Ocewan Circulation Experiment (WOCE) and the study of thew Tropical Ocean and the Global Atmosphere (TOGA).